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Super Mario 64, Super Smash Bros, Goldeneye, if you like Star Wars Shadows of the Empire is great. Top Gear Rally is great. Star Wars Episode 1: Racer is pretty sweet as well. Not easy though!
The second bond game for N64 is much better IMO but goldeneye was great until then. Perfect Dark is great as well. I have a ton of games for it still and can't remember most of them. Another fun game if I remember right was Sarges Heroes, you're a plastic army man and the multiplayer was really fun.
Mario kart is a great game no matter how old you are. Perfect dark is a little better for older people, but a sweet game (hope you have a memory card) and goldeneye is also awesome. Now that I have thrown off games that people have already mentioned...
What about NFL Blitz? that game was quite fun (and there are TONS of cheats that you can find online)
well they already said my fav. 007 sweet multiplay also like the spinoff perfect dark, mario kart, mario 64. like someone already said go to funcoland, ebgames, or where ever that they sale used games
I'll second Conker's Bad Fur Day. And I'll throw in "Off Road Challenge". Not a whole lot to that game, but it'll easily waste a whole day. I should go look at a second hand game store today.
Starfox 64 is a good one for the kids, and you may like it yourself. RUSH 2 is a great racing game, and Turok 2: seeds of evil is pretty good for the mature people.